Double resonance spectroscopy of phenol(H2O)1–12: evidence for ice-like structures in aromate–water clusters?
Identifieur interne : 000C39 ( Main/Exploration ); précédent : 000C38; suivant : 000C40Double resonance spectroscopy of phenol(H2O)1–12: evidence for ice-like structures in aromate–water clusters?
Auteurs : W. Roth [Allemagne] ; M. Schmitt [Allemagne] ; Ch Jacoby [Allemagne] ; D. Spangenberg [Allemagne] ; Ch Janzen [Allemagne] ; K. Kleinermanns [Allemagne]Source :
- Chemical Physics [ 0301-0104 ] ; 1997.
Abstract
Phenol(H2O)n clusters have been studied in the electronic ground state by dispersed fluorescence spectroscopy and in the electronically excited state by means of two-color resonant two-photon ionization (R2PI), spectral hole burning and rotationally resolved laser-induced fluorescence. Resonant spectra up to a cluster size of n=12 have been obtained by two-color R2PI under `soft' ionization conditions. The analysis of spectral shifts and of the intermolecular vibrations in both electronic states is used to assign structures for these bi-, tri- and (partially) tetracoordinated hydrogen bonded systems, which may be comparable to H-bond-deficient water structures at the surface of liquid water and ice.
Url:
DOI: 10.1016/S0301-0104(98)00252-3
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Resonant spectra up to a cluster size of n=12 have been obtained by two-color R2PI under `soft' ionization conditions. The analysis of spectral shifts and of the intermolecular vibrations in both electronic states is used to assign structures for these bi-, tri- and (partially) tetracoordinated hydrogen bonded systems, which may be comparable to H-bond-deficient water structures at the surface of liquid water and ice.</div></front></TEI><affiliations><list><country><li>Allemagne</li></country><region><li>District de Düsseldorf</li><li>Rhénanie-du-Nord-Westphalie</li></region><settlement><li>Düsseldorf</li></settlement></list><tree><country name="Allemagne"><region name="Rhénanie-du-Nord-Westphalie"><name sortKey="Roth, W" sort="Roth, W" uniqKey="Roth W" first="W" last="Roth">W. 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